Dielectric nanostructures are cherished because of their great potential for low-loss optical devices. Achieving strong optical resonances in dielectric nanostructures is the key to realizing practical dielectric metadevices. In particular, the exploration of new mechanisms for high quality (Q) factor resonances in dielectric architectures provides the basis for actively tunable responses and nonlinearities. In this work, we study the switchable optical responses from dielectric/plasmonic hybrid systems and the nonlinearities in pure dielectric nanostructures supporting optical resonances associated with the bound states in the continuum (BICs). First, we show that, under optical excitations, hybrid metasurfaces based on a dielectric nanoantenna array of active materials (such as silicon (Si) and zinc oxide (ZnO)) on a plasmonic (e.g., silver (Ag)) backplane exhibit broadly tunable topological properties. Accordingly, enormously strong polarization manipulation of near-infrared light in the vicinity of the topological features is observed. Second, we study the efficient second harmonic generation (SHG) from asymmetric lithium niobate (LN) metasurfaces. Third, based on the large Kerr nonlinearities of silicon, we explore the nonlinear chiroptical response from a planar Si metasurface supporting high Q-factor guided mode resonances (GMRs) at near-infrared wavelengths. Fourth, leveraging the momentum-space polarization vortices observed in photonic structures, we investigate the switchable and nonlinear optical vortex generation from Si photonic crystal slabs. Our work shows that dielectric nanostructures which support high-Q resonances via careful nanoengineering can serve as a transformative platform for active and nonlinear photonics.
Optical vortices, the spatial modes of an electromagnetic wave carrying orbital angular momentum (OAM), have attracted increasing interest because of their potential for applications in optical communication with enhanced security and channel capacity. A unique optical vortex (OV) generation method has been recently proposed based on the Pancharatnam–Berry (PB) phase induced by the winding topology of polarization around a vortex singularity at bound states in the continuum (BIC). Compared with the recently emergent metasurface-based OV generators, which rely on spatial variations, the BIC-based OV generators have yielded advances in terms of design feasibility, fabrication complexity, and robustness. However, their applications in practical photonic systems are currently limited because OV generations from BIC-related devices originate from the topological property of the photonic bands and cannot be dynamically altered. Here, by leveraging the vortex topology in momentum space together with the nonlinear dynamics of silicon, we demonstrate that a silicon photonic crystal slab can realize optically switchable OV generation. In particular, the spatial tunability and the switching effects in the picosecond scale are studied using nonlinear modeling at near-infrared wavelengths. The demonstrated nontrivial topological nature of the active generators can expand the application of BIC-based devices to include ultrafast vortex beam generation, high-capacity optical communication, and mode-division multiplexing.
dWe demonstrate a nonlinear chiral meta-mirror consisting of an array of amorphous silicon split-ring resonators on top of a silver backplane with a silica spacer layer. This hybrid dielectric-plasmonic system can enhance Mie-resonance to result in strong light-matter interaction on the nanometer scale. The chiral meta-mirror exhibits a sharp absorption on one handedness of the circular polarization, and reflects the opposite handedness in a manner that preserves its polarization state in the linear regime. We show that the chiroptical responses can be tuned dynamically by leveraging photoexcited carriers in amorphous silicon. All optical, picosecond scale intensity modulation and polarization switching are studied.
The dramatic optical property change of optical phase change materials (O-PCMs) allows the realization of tunable optical and photonic devices with enhanced optical functionalities, such as reconfigurable optics, optical switches and routers, and photonic memories. Recently we developed a new class of non-volatile O-PCM, Ge-Sb-Se-Te (GSST), which features unprecedented broadband optical transparency (1-18.5 micron), large optical contrast (dn = 2) and significantly improved glass forming ability. Leveraging the remarkable material property and advanced design methods, we develop a suite of reconfigurable, all-dielectric metasurface optics with unprecedented performance. In one example, a focal length tunable transmissive metalens is demonstrated showing diffraction-limited imaging performance and complete optical function switching during the phase transition, which sets the foundation for ultra-compact, solid-state, tunable meta-optical systems.
The unique light-matter interaction in metamaterials, a type of artificial medium in which the geometrical features of subunits dominate their optical responses, have been utilized to achieve exotic material properties that are rare or nonexistent in natural materials. Furthermore, to extend their behaviors, active materials have been introduced into metamaterial systems to advance tunability, switchability and nonlinearity. Nevertheless, practical examples of versatile photonic metamaterials remain exceedingly rare for two main reasons. On the one hand, in sharp contrast to the broad material options available at lower frequencies, it is less common to find active media in the optical regime that can provide pronounced dielectric property changes under external stimuli, such as electric and magnetic fields. Vanadium dioxide (VO2), offering a large refractive index variation over a broad frequency range due to its near room temperature insulator-to-metal transition (IMT), has been favored in recent studies on tunable metamaterials. On the other hand, it turns out that regulating responses of hybrid metamaterials to external forces in an integrated manner is not a straightforward task. Recently, metamaterial-enabled devices (i.e., metadevices) with ‘self-sufficient’ or ‘self-contained’ electrical and optical properties have enabled complex functionalities. Here, we present a design methodology along with the associated experimental validation of a VO2 thin film integrated optical metamaterial absorber as a hybrid photonic platform for electrically driven multifunctional control, including reflectance switching, a rewritable memory process and manageable localized camouflage. The nanoengineered topologically continuous metal structure simultaneously supports the optical resonance and electrical functionality that actuates the phase transition in VO2 through the process of Joule heating. This work provides a universal approach to creating self-sufficient and highly-versatile nanophotonic systems.
Nanostructured metals have utilized the strong spatial confinement of surface plasmon polaritons to harness enormous energy densities on their surfaces, and have demonstrated vast potential for the future of nano-optical systems and devices. While the spectral location of the plasmonic resonance can be tailored with relative ease, the control over the spectral linewidth associated with loss represents a more daunting task. In general, plasmonic resonances typically exhibit a spectral linewidth of ~50 nm, limited largely by the combined damping and radiative loss in nanometallic structures. Here, we present one of the sharpest resonance features demonstrated by any plasmonic system reported to date by introducing dark plasmonic modes in diatomic gratings. Each duty cycle of the diatomic grating consists of two nonequivalent metallic stripes, and the asymmetric design leads to the excitation of a dark plasmonic mode under normal incidence. The dark plasmonic mode in our structure, occurring at a prescribed wavelength of ~840 nm, features an ultra-narrow spectral linewidth of about 5 nm, which represents a small fraction of the value commonly seen in typical plasmonic resonances. We leverage the dark plasmonic mode in the metallic nanostructure and demonstrate a resonance enhanced plasmoelectric effect, where the photon-induced electric potential generated in the grating is shown to follow the resonance behavior in the spectral domain. The light concentrating ability of dark plasmonic modes in conjunction with the ultra-sharp resonance feature at a relatively low loss offers a novel route to enhanced light-matter interactions with high spectral sensitivity for diverse applications.
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